文献类型：期刊文献

英文题名：Electrocatalyst design strategies for ammonia production via N2 reduction

作者：Li, Ziwei Li, Min Yang, Jiachen Liao, Mingyue Song, Guoqiang Cao, Jianxin Liu, Fei Wang, Zhigang Kawi, Sibudjing Lin, Qian

第一作者：Li, Ziwei

通信作者：Song, Guoqiang

机构：[1] School of Chemistry and Chemical engineering, Guizhou Provincial Key Laboratory of Green Chemical and Clean Energy Technology, Guizhou University, Guiyang, 550025, China; [2] School of Civil Engineering, Guizhou Institute of Technology, Guiyang, 550003, China; [3] School of Chemical Engineering, Guizhou Institute of Technology, Guiyang, 550003, China; [4] Department of Chemical and Biomolecular Engineering, National University of Singapore, Singapore, 117585, Singapore

第一机构：School of Chemistry and Chemical engineering, Guizhou Provincial Key Laboratory of Green Chemical and Clean Energy Technology, Guizhou University, Guiyang, 550025, China

通信机构：School of Chemical Engineering, Guizhou Institute of Technology, Guiyang, 550003, China|贵州理工学院化学工程学院;贵州理工学院;

年份：2022

卷号：388-389

起止页码：12-25

外文期刊名：Catalysis Today

收录：EI(收录号：20212610562092);Scopus(收录号：2-s2.0-85108541198)

语种：英文

外文关键词：Energy efficiency - Design - Electronic structure - Electrolytic reduction - Electrolysis - Ammonia

摘要：Ammonia production via N2 activation and electroreduction under ambient conditions has triggered considerable interests because it is a cleaner and more sustainable process compared with the traditional Haber-Bosch process. Designing efficient electrocatalysts is crucial to solve the inherent low energy efficiency issue of N2 reduction reaction (NRR) to sustainably produce NH3. This review summarizes the recent progress in design strategies of efficient NRR electrocatalysts including electronic structure tuning to enhance the intrinsic activity and active sites exposuring to improve the apparent activity. Further, experimental protocols to achieve reliable NRR results are also discussed and proposed. This review is expected to inspire novel electrocatalysts design to promote the NRR research field. ? 2021