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Process simulation of coal-direct chemical looping gasification for syngas production  ( SCI-EXPANDED收录 EI收录)   被引量:6

文献类型:期刊文献

英文题名:Process simulation of coal-direct chemical looping gasification for syngas production

作者:Liu, Lang Cao, Yan Ma, Dongran Liu, Qingcai Yang, Jian

第一作者:刘浪

通信作者:Liu, L[1];Cao, Y[2]

机构:[1]Guizhou Inst Technol, Chem Engn Inst, Guiyang 550003, Guizhou, Peoples R China;[2]Western Kentucky Univ, Dept Chem, Inst Combust Sci & Environm Technol, Bowling Green, KY 42101 USA;[3]Chongqing Univ, Coll Mat Sci & Engn, Chongqing 400044, Peoples R China

第一机构:贵州理工学院

通信机构:corresponding author), Guizhou Inst Technol, Chem Engn Inst, Guiyang 550003, Guizhou, Peoples R China;corresponding author), Western Kentucky Univ, Dept Chem, Inst Combust Sci & Environm Technol, Bowling Green, KY 42101 USA.|贵州理工学院;

年份:2017

卷号:7

期号:87

起止页码:55450-55458

外文期刊名:RSC ADVANCES

收录:;EI(收录号:20181404975880);Scopus(收录号:2-s2.0-85044671212);WOS:【SCI-EXPANDED(收录号:WOS:000418378100064)】;

基金:This study was supported by the Youth Science and Technology Talents Growth project of the Guizhou Provincial Education Department (Qianjiaohe KY Zi [2017]220), and the Energy Chemistry Laboratory in Guizhou Province (Qianjiaohe KY Zi [2017]009).

语种:英文

外文关键词:Carbon - Coal - Free energy - Gibbs free energy - Synthesis gas - Synthesis gas manufacture

摘要:The coal gasification process is used in the commercial production of syngas as a means toward the clean use of coal. In this paper, the process of syngas production via the coal-direct chemical looping gasification process (CDCLG) is modeled under thermochemical equilibrium with the Gibbs free energy approach, and the model is developed using a complete and comprehensive simulation model. Due to the kinetic limits of char gasification, the carbon conversion efficiency is not suggested to be larger than 0.9 in the fuel reactor during the CDCLG process. Besides, the simulation results suggest the residual carbon should be burnt in the air reactor. Moreover, the effects of various conditions, which include carbon conversion, temperature, pressure and the steam feed ratio, on the input and energy output parameters, including the air feed ratio, efficiency of electricity and syngas quality, are studied and revealed in this paper.

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