文献类型：期刊文献

英文题名：Electrocatalyst design strategies for ammonia production via N-2 reduction

作者：Li, Ziwei Li, Min Yang, Jiachen Liao, Mingyue Song, Guoqiang Cao, Jianxin Liu, Fei Wang, Zhigang Kawi, Sibudjing Lin, Qian

第一作者：Li, Ziwei

通信作者：Lin, Q[1];Song, GQ[2];Kawi, S[3]

机构：[1]Guizhou Univ, Sch Chem & Chem Engn, Guizhou Prov Key Lab Green Chem & Clean Energy Te, Guiyang 550025, Peoples R China;[2]Guizhou Inst Technol, Sch Civil Engn, Guiyang 550003, Peoples R China;[3]Guizhou Inst Technol, Sch Chem Engn, Guiyang 550003, Peoples R China;[4]Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore

第一机构：Guizhou Univ, Sch Chem & Chem Engn, Guizhou Prov Key Lab Green Chem & Clean Energy Te, Guiyang 550025, Peoples R China

通信机构：corresponding author), Guizhou Univ, Sch Chem & Chem Engn, Guizhou Prov Key Lab Green Chem & Clean Energy Te, Guiyang 550025, Peoples R China;corresponding author), Guizhou Inst Technol, Sch Chem Engn, Guiyang 550003, Peoples R China;corresponding author), Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore.|贵州理工学院化学工程学院;贵州理工学院;

年份：2022

卷号：388-389

起止页码：12-25

外文期刊名：CATALYSIS TODAY

收录：;WOS:【SCI-EXPANDED(收录号:WOS:000760340300003)】；

基金：This work was supported by Natural Science Foundation of Guizhou University for Specially Contracted Professors (GDTGHZ(201905)), Science and Technology Supporting Foundation of Liupanshui (52020-2018-01-04, H2020-003, K21-0114-025), Scientific and Technological Innovation Talents Team Project of Guizhou Province (No. 20185607), National Natural Science Foundation of China (22062003), and the Natural Science Foundation of Guizhou ([2019]2872 and [2020] 1Y037).

语种：英文

外文关键词：Electrochemical N-2 reduction; Electrocatalyst; Design strategy; Experimental protocol

摘要：Ammonia production via N-2 activation and electroreduction under ambient conditions has triggered considerable interests because it is a cleaner and more sustainable process compared with the traditional Haber-Bosch process. Designing efficient electrocatalysts is crucial to solve the inherent low energy efficiency issue of N-2 reduction reaction (NRR) to sustainably produce NH3. This review summarizes the recent progress in design strategies of efficient NRR electrocatalysts including electronic structure tuning to enhance the intrinsic activity and active sites exposuring to improve the apparent activity. Further, experimental protocols to achieve reliable NRR results are also discussed and proposed. This review is expected to inspire novel electrocatalysts design to promote the NRR research field.